Steve Rogers / Captain America

Nick Fury

Natasha Romanoff / Black Widow

Alexander Pierce

Bucky Barnes / Winter Soldier

Sam Wilson / Falcon

Maria Hill

Brock Rumlow

Jasper Sitwell

Kate / Agent 13

Peggy Carter

Dr. Arnim Zola

Smithsonian Guard

Jack Rollins

Councilwoman Hawley

Councilman Singh

Councilman Rockwell

Councilman Yen

Senator Stern

Georges Batroc

French Pirate #1

French Pirate #2

Engine Pirate

French Radio Pirate

Skinny Steve

Launch Tech #1

Launch Tech #2

Dr. Fine

SHIELD Interrogator #1

SHIELD Interrogator #2

Scientist #1

Scientist #2

Apple Employee

Com Tech #1

Com Tech #2

Renata

Garcia

Charlie XO

Charlie Weapons Tech

SHIELD Tech

Lead SHIELD Pilot

Senior SHIELD Agent

SHIELD Agent

Strike SGT. #1

Strike SGT. #2

Strike Agent

Strike Agent

Strike Agent

Strike Agent

25ᵗʰ Floor Strike Agent

Scudder

Human Resources Executive

Doctor

Lead EMT

CIA Instructor

Capitol Hill Police

Capitol Hill Police

FBI Agent

FBI Agent

Committee Member

Little Boy in the Smithsonian

Fury Car Voice (voice)

SHIELD Computer (voice)

The Smithsonian Narrator (voice)

Dr. List (uncredited)

SHIELD Agent (uncredited)

Museum Visitor (uncredited)

Baron Wolfgang von Strucker (uncredited)

Wanda Maximoff / Scarlet Witch (uncredited)

Committee General (uncredited)

Pietro Maximoff / Quicksilver (uncredited)

Man on Escalator in Museum (uncredited)

Smithsonian Museum Visitor

Writing

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Sound

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Editing

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